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The Lost Patrol
While you're wandering outside Boston, you may pick up a strange distress call. If you investigate, you'll run into a whole bunch of Super Mutants that need dealing with. Once you've done that, you'll find that the signal is coming from a dead Brotherhood of Steel scribe. Listen to his holotape, and learn how he died. You'll then be able to track down the other members of his squad, all of whom have met their end in various ways. The final step will be to confront the lone survivor - the Paladin that's gone quite mad and locked himself inside a bunker. How you decide to deal with him is completely up to you.